Skip to content
naulon

No retraction, correction or concern found when last checked on Oct 25, 2026.

Photonic-crystal exciton-polaritons in monolayer semiconductors

Long Zhang, Rahul Gogna, Will Burg and 2 more

Nature Communications · 2018 · CC BY

doi:10.1038/s41467-018-03188-x

Abstract

Semiconductor microcavity polaritons, formed via strong exciton-photon coupling, provide a quantum many-body system on a chip, featuring rich physics phenomena for better photonic technology. However, conventional polariton cavities are bulky, difficult to integrate, and inflexible for mode control, especially for room-temperature materials. Here we demonstrate sub-wavelength-thick, one-dimensional photonic crystals as a designable, compact, and practical platform for strong coupling with atomically thin van der Waals crystals. Polariton dispersions and mode anti-crossings are measured up to room temperature. Non-radiative decay to dark excitons is suppressed due to polariton enhancement of the radiative decay. Unusual features, including highly anisotropic dispersions and adjustable Fano resonances in reflectance, may facilitate high temperature polariton condensation in variable dimensions. Combining slab photonic crystals and van der Waals crystals in the strong coupling regime allows unprecedented engineering flexibility for exploring novel polariton phenomena and device concepts.

Full text

Its licence does not allow us to show the full text. Read it at PubMed Central:

Read at PubMed Central

References 54

  1. 1.

    Deng H, Haug H, Yamamoto Y. Exciton-polariton Bose-Einstein condensation. Rev. Mod. Phys. 2010;82:1489-1537.

    Not in our library10.1103/revmodphys.82.1489

  2. 2.

    Carusotto I, Ciuti C. Quantum fluids of light. Rev. Mod. Phys. 2013;85:299-366.

    Not in our library10.1103/revmodphys.85.299

  3. 3.

    Fraser MD, Hofling S, Yamamoto Y. Physics and applications of exciton-polariton lasers. Nat. Mater. 2016;15:1049-1052.

    Not in our library10.1038/nmat4762

  4. 4.

    Karzig T, Bardyn CE, Lindner NH, Refael G. Topological polaritons. Phys. Rev. X. 2015;5:031001.

    Not in our library

  5. 5.

    Bardyn CE, Karzig T, Refael G, Liew TCH. Topological polaritons and excitons in garden-variety systems. Phys. Rev. B. 2015;91:161413(R).

    Not in our library10.1103/physrevb.91.161413

  6. 6.

    Nalitov A, Malpuech G, Teras H, Solnyshkov D. Spin-orbit coupling and the optical spin hall effect in photonic graphene. Phys. Rev. Lett. 2015;114:026803.

    Not in our library10.1103/physrevlett.114.026803

  7. 7.

    Liew TCH, Kavokin AV, Shelykh IA. Optical circuits based on polariton neurons in semiconductor microcavities. Phys. Rev. Lett. 2008;101:016402.

    Not in our library10.1103/physrevlett.101.016402

  8. 8.

    Liew TCH, Savona V. Single photons from coupled quantum modes. Phys. Rev. Lett. 2010;104:183601.

    Not in our library10.1103/physrevlett.104.183601

  9. 9.

    Flayac H, Savona V. Single photons from dissipation in coupled cavities. Phys. Rev. A. 2016;94:013815.

    Not in our library10.1103/physreva.94.013815

  10. 10.

    Joana C, van Loock P, Deng H, Byrnes T. Steady-state generation of negative-Wigner-function light using feedback. Phys. Rev. A. 2016;94:063802.

    Not in our library10.1103/physreva.94.063802

  11. 11.

    Byrnes T, Recher P, Yamamoto Y. Mott transitions of exciton polaritons and indirect excitons in a periodic potential. Phys. Rev. B. 2010;81:205312.

    Not in our library10.1103/physrevb.81.205312

  12. 12.

    Douglas JS, et al. Quantum many-body models with cold atoms coupled to photonic crystals. Nat. Photonics. 2015;9:326-331.

    Not in our library10.1038/nphoton.2015.57

  13. 13.

    Angelakis, D. G. Quantum Simulations with Photons and Polaritons (Springer, 2017).

    Not in our library

  14. 14.

    Mak KF, Lee C, Hone J, Shan J, Heinz TF. Atomically thin MoS2: a new direct-gap semiconductor. Phys. Rev. Lett. 2010;105:136805.

    Not in our library10.1103/physrevlett.105.136805

  15. 15.

    Splendiani A, et al. Emerging photoluminescence in monolayer MoS2. Nano Lett. 2010;10:1271-1275.

    Not in our library10.1021/nl903868w

  16. 16.

    Geim AK, Grigorieva IV. Van der Waals heterostructures. Nature. 2013;499:419-425.

    Not in our library10.1038/nature12385

  17. 17.

    Liu X, et al. Strong lightmatter coupling in two-dimensional atomic crystals. Nat. Photonics. 2014;9:30-34.

    Not in our library10.1038/nphoton.2014.304

  18. 18.
  19. 19.

    Sidler M, et al. Fermi polaron-polaritons in charge-tunable atomically thin semiconductors. Nat. Phys. 2016;13:255-261.

    Not in our library10.1038/nphys3949

  20. 20.

    Flatten LC, et al. Room-temperature exciton-polaritons with two-dimensional WS2. Sci. Rep. 2016;6:33134.

    Not in our library10.1038/srep33134

  21. 21.

    Liu X, et al. Control of coherently coupled exciton polaritons in monolayer tungsten disulphide. Phys. Rev. Lett. 2017;119:027403.

    Not in our library10.1103/physrevlett.119.027403

  22. 22.

    Chen YJ, Cain JD, Stanev TK, Dravid VP, Stern NP. Valley-polarized exciton-polaritons in a monolayer semiconductor. Nat. Photonics. 2017;11:431-435.

    Not in our library10.1038/nphoton.2017.86

  23. 23.

    Dufferwiel S, et al. Valley-addressable polaritons in atomically thin semiconductors. Nat. Photonics. 2017;11:497-501.

    Not in our library10.1038/nphoton.2017.125

  24. 24.

    Sercombe D, et al. Optical investigation of the natural electron doping in thin MoS2 films deposited on dielectric substrates. Sci. Rep. 2013;3:3489.

    Not in our library10.1038/srep03489

  25. 25.

    Wang S, et al. Coherent coupling of WS2 monolayers with metallic photonic nanostructures at room temperature. Nano Lett. 2016;16:4368-4374.

    Not in our library10.1021/acs.nanolett.6b01475

  26. 26.

    Liu W, et al. Strong exciton–plasmon coupling in MoS2 coupled with plasmonic lattice. Nano Lett. 2016;16:1262-1269.

    Not in our library10.1021/acs.nanolett.5b04588

  27. 27.

    Lundt N, et al. Room-temperature Tamm-plasmon exciton-polaritons with a WSe2 monolayer. Nat. Commun. 2016;7:13328.

    Not in our library10.1038/ncomms13328

  28. 28.

    Sun Z, et al. Optical control of room-temperature valley polaritons. Nat. Photonics. 2017;11:491-496.

    Not in our library10.1038/nphoton.2017.121

  29. 29.

    Bhanu U, Islam MR, Tetard L, Khondaker SI. Photoluminescence quenching in gold - MoS2 hybrid nanoflakes. Sci. Rep. 2015;4:5575.

    Not in our library10.1038/srep05575

  30. 30.

    Dalfovo F, Giorgini S, Pitaevskii LP, Stringari S. Theory of Bose-Einstein condensation in trapped gases. Rev. Mod. Phys. 1999;71:463-512.

    Not in our library10.1103/revmodphys.71.463

  31. 31.

    ODonnell KP, Chen X. Temperature dependence of semiconductor band gaps. Appl. Phys. Lett. 1991;58:2924-2926.

    Not in our library10.1063/1.104723

  32. 32.

    Rudin S, Reinecke TL. Temperature-dependent exciton linewidths in semiconductor quantum wells. Phys. Rev. B. 1990;41:3017.

    Not in our library10.1103/physrevb.41.3017

  33. 33.

    Zhang XX, You Y, Zhao SYF, Heinz TF. Experimental evidence for dark excitons in monolayer WSe2. Phys. Rev. Lett. 2015;115:257403.

    Not in our library10.1103/physrevlett.115.257403

  34. 34.

    Wang G, et al. Spin-orbit engineering in transition metal dichalcogenide alloy monolayers. Nat. Commun. 2015;6:10110.

    Not in our library10.1038/ncomms10110

  35. 35.

    Zhou W, et al. Progress in 2d photonic crystal Fano resonance photonics. Progress Quantum Electron. 2014;38:1-74.

    Not in our library10.1016/j.pquantelec.2014.01.001

  36. 36.

    Miroshnichenko AE, Flach S, Kivshar YS. Fano resonances in nanoscale structures. Rev. Mod. Phys. 2010;82:2257-2298.

    Not in our library10.1103/revmodphys.82.2257

  37. 37.

    Wang, Y. et al. Exciton-polariton Fano resonance driven by second harmonic generation. Phys. Rev. Lett.118, 063602 (2017).

    Not in our library10.1103/physrevlett.118.063602

  38. 38.

    Savvidis PG, et al. Angle-resonant stimulated polariton amplifier. Phys. Rev. Lett. 2000;84:1547-1547.

    Not in our library10.1103/physrevlett.84.1547

  39. 39.

    Deng H, Weihs G, Snoke D, Bloch J, Yamamoto Y. Polariton lasing vs. photon lasing in a semiconductor microcavity. Proc. Natl Acad. Sci. USA. 2003;100:15318-15323.

    Not in our library10.1073/pnas.2634328100

  40. 40.

    Amo A, et al. Excitonpolariton spin switches. Nat. Photonics. 2010;4:361-366.

    Not in our library10.1038/nphoton.2010.79

All 54 references

Cited by papers we hold 2

Reads

Read by people on this page

None yet.

Checked or read by AI through naulon

None yet.

A person counts once a day per paper. We keep no cookie and no address: a reader is a hash that changes every day. Any month under five reads shows no number.

Are you an author?

Is this your paper?

Claim it to add your note and be paid when agents cite it. Free.