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High-Performance Membrane Capacitive Deionization Based on Metal−Organic Framework-Derived Hierarchical Carbon Structures

Wenhui Shi, Chenzeng Ye, Xilian Xu and 7 more

ACS Omega · 2018

doi:10.1021/acsomega.8b01356 (opens in a new tab)

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Abstract

Membrane capacitive deionization (MCDI) is a simple and highly energy efficient method to convert brackish water to clean water. In this work, a high-performance MCDI electrode architecture, which is composed of three-dimensional graphene networks and metal–organic frameworks (MOFs)–derived porous carbon rods, was prepared by a facile method. The obtained electrode material possesses not only the conducting networks for rapid electron transport but also the short diffusion length of ions, which exhibits excellent desalination performance with a high salt removal capacity, i.e., 37.6 mg g–1 at 1.2 V in 1000 mg L–1 NaCl solution. This strategy can be extended to other MOF-derived MCDI electrodes.

Abstract licence: CC BY-NC-ND

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