Defect‐Engineered Metal–Organic Frameworks

Abstract

Defect engineering in metal–organic frameworks (MOFs) is an exciting concept for tailoring material properties, which opens up novel opportunities not only in sorption and catalysis, but also in controlling more challenging physical characteristics such as band gap as well as magnetic and electrical/conductive properties. It is challenging to structurally characterize the inherent or intentionally created defects of various types, and there have so far been few efforts to comprehensively discuss these issues. Based on selected reports spanning the last decades, this Review closes that gap by providing both a concise overview of defects in MOFs, or more broadly coordination network compounds (CNCs), including their classification and characterization, together with the (potential) applications of defective CNCs/MOFs. Moreover, we will highlight important aspects of “defect‐engineering” concepts applied for CNCs, also in comparison with relevant solid materials such as zeolites or COFs. Finally, we discuss the future potential of defect‐engineered CNCs.

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     Kim M, Cahill JF, Su YX, Prather KA, Cohen SM. Chem. Sci. 2012;3:126-130.

     Not in our library

126. 126.

     Karagiaridi O, Bury W, Mondloch JE, Hupp JT, Farha OK. Angew. Chem. Int. Ed. 2014;53:4530-4540.

     Not in our library10.1002/anie.201306923

127. 127.

     Li T, Kozlowski MT, Doud EA, Blakely MN, Rosi NL. J. Am. Chem. Soc. 2013;135:11688-11691.

     Not in our library10.1021/ja403810k

128. 128.

     Brozek CK, Dinca M. J. Am. Chem. Soc. 2013;135:12886-12891.

     Not in our library10.1021/ja4064475

129. 129.

     Lalonde M, Bury W, Karagiaridi O, Brown Z, Hupp JT, Farha OK. J. Mater. Chem. A. 2013;1:5453-5468.

     Not in our library

130. 130.

     Ameloot R, Aubrey M, Wiers BM, Gomora-Figueroa AP, Patel SN, Balsara NP, Long JR. Chem. Eur. J. 2013;19:5533-5536.

     Not in our library10.1002/chem.201300326

131. 131.

     Hendon CH, Tiana D, Walsh A. Phys. Chem. Chem. Phys. 2012;14:13120-13132.

     Not in our library10.1039/c2cp41099k

132. 132.

     Talin AA, Centrone A, Ford AC, Foster ME, Stavila V, Haney P, Kinney RA, Szalai V, El Gabaly F, Yoon HP, Léonard F, Allendorf MD. Science. 2014;343:66-69.

     Not in our library10.1126/science.1246738

133. 133.

     Sheberla D, Sun L, Blood-Forsythe MA, Er S, Wade CR, Brozek CK, Aspuru-Guzik A, Dinc M. J. Am. Chem. Soc. 2014;136:8859-8862.

     Not in our library10.1021/ja502765n

Cited by papers we hold 9

• Mechanochemically Synthesized Prussian Blue for Efficient Removal of Cesium Ions from Aqueous Solutions · 2022
  Not checked
• Metal-Organic Frameworks: Synthetic Methods and Potential Applications · 2021
  No notice
• Modulated self-assembly of metal–organic frameworks · 2020
  No notice
• Metal–organic framework gels and monoliths · 2020
  No notice
• Multivariate Modulation of the Zr MOF UiO‐66 for Defect‐Controlled Combination Anticancer Drug Delivery · 2020
  No notice
• A coronene-based semiconducting two-dimensional metal-organic framework with ferromagnetic behavior · 2018
  No notice
• Curved crystal morphology, photoreactivity and photosalient behaviour of mononuclear Zn(II) complexes · 2017
  Not checked
• Metal–organic and covalent organic frameworks as single-site catalysts · 2017
  No notice
• Construction of hierarchically porous metal–organic frameworks through linker labilization · 2017
  No notice

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